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- Transport of dipolar excitons in (Al,Ga)N/GaN quantum wells. doi link

Auteur(s): Fedichkin F., Andreakou P., Jouault B., Vladimirova M., Guillet T., Brimont C., Valvin P., Bretagnon T., Dussaigne Amélie, Grandjean Nicolas, Lefebvre P.

(Article) Publié: -Physical Review B Condensed Matter And Materials Physics (1998-2015), vol. 91 p.205424 (2015)
Texte intégral en Openaccess : arxiv


Ref HAL: hal-01154792_v1
DOI: 10.1103/PhysRevB.91.205424
WoS: 000354972700012
Exporter : BibTex | endNote
19 Citations
Résumé:

We investigate the transport of dipolar indirect excitons along the growth plane of polar (Al,Ga)N/GaN quantum well structures by means of spatially and time-resolved photoluminescence spectroscopy. The transport in these strongly disordered quantum wells is activated by dipole-dipole repulsion. The latter induces an emission blue shift that increases linearly with exciton density, whereas the radiative recombination rate increases exponentially. Under continuous, localized excitation, we observe continuously decreasing emission energy, as excitons propagate away from the excitation spot. This corresponds to a steady-state gradient of exciton density,measured over several tens of micrometers. Time-resolved microphotoluminescence experiments provide information on the dynamics of recombination and transport of dipolar excitons.We account for the ensemble of experimental results by solving the nonlinear drift-diffusion equation. Quantitative analysis suggests that in such structures, exciton propagation on the scale of 10 to 20 μm is mainly driven by diffusion, rather than by drift, due to the strong disorder and the presence of nonradiative defects. Secondary exciton creation, most probably by the intense higher-energy luminescence, guided along the sample plane, is shown to contribute to the excitonemission pattern on the scale up to 100 μm. The exciton propagation length is strongly temperature dependent, the emission being quenched beyond a critical distance governed by nonradiative recombination.