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- Transport of indirect excitons in GaN quantum wells. hal link

Auteur(s): Guillet T., Jouault B., Fedichkin F., Lefebvre P., Brimont C., Valvin P., Bretagnon T., Lahourcade Lise, Grandjean N., Vladimirova M.

Conference: International Workshop on Nitride Semiconductors (IWN 2016) (Orlando, US, 2016-10-02)


Ref HAL: hal-01388983_v1
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Résumé:

Excitons in nitride quantum wells (QWs) are naturally indirect due to the strong internal electric field: electron and hole within such excitons are spatially separated, leading to strong dipole moments and long radiative lifetimes. Extensive studies of indirect excitons (IXs) in GaAs-based heterostructures have shown that a combination of these two features results in many interesting properties of IXs: they can propagate over large distances, can be controlled in-situ by light and external gate voltage, cool down to the lattice temperature before recombination, and form cold and dense gas of interacting bosons. Compared to traditional IXs in arsenide heterostrutures, IXs in GaN QWs have much larger binding energies and smaller Bohr radii. This allows exploring IX propagation up to room temperature, and over a much larger density range. Using spatially- and time-resolved photoluminescence experiments, we have investigated the exciton transport in a 7 nm-wide GaN single QW sandwiched between Al0.19Ga0.81N barriers. The IX emission is imaged, with spectral and temporal resolutions, along the sample plane. Therefore the corresponding spatial density profiles are obtained and monitored as a function of (i) temperature, (ii) the exciton density at the excitation spot, (iii) the substrate material (GaN vs Sapphire) and (iv) the excitation regime (continuous vs pulsed excitation) [F. Fedichkin et al., Phys. Rev. B 91, 205424 (2015)]. We provide a comprehensive analysis of the data combined with numerical modeling, and we show that the efficient propagation of IXs takes place in the high density regime where the in-plane disorder is efficiently screened by the dipole-dipole interaction. Under these latter conditions, exciton mobility is almost temperature-independent from 10K up to room temperature. This suggests that exciton-exciton interaction is by far the dominant scattering mechanism, compared to scattering by the interface disorder. However, the exciton transport is maintained up to 300K only in the QW that was epitaxially grown on a GaN substrate, since nonradiative processes dominate the transport in the case of a sapphire substrate, for which high densities of threading dislocations are present.We provide a detailed understanding of the physical mechanisms of IX transport and its temperature and density dependence, and we show that nitride-hosted IXs constitute a promising system for the formation of collective bosonic states in semiconductors. Financial support: projects INDEX (FP7 PITN-GA-2011-289968) and OBELIX (ANR-15-CE30-0020-02).