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Physique Statistique
(37) Production(s) de l'année 2019
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Hierarchical landscape of hard disk glasses
Auteur(s): Liao Qinyi, Berthier L.
(Article) Publié:
Physical Review X, vol. 9 p.011049 (2019)
Texte intégral en Openaccess :
Ref HAL: hal-02092636_v1
Ref Arxiv: 1810.10256
DOI: 10.1103/PhysRevX.9.011049
WoS: 000461916500001
Ref. & Cit.: NASA ADS
Exporter : BibTex | endNote
9 Citations
Résumé: We numerically analyse the landscape governing the evolution of the vibrational dynamics of hard disk glasses as the density increases towards jamming. We find that the dynamics becomes slow, spatially correlated, and starts to display aging dynamics across an avoided Gardner transition, with a phenomenology that resembles three dimensional observations. We carefully analyse the behaviour of single glass samples, and find that the emergence of aging dynamics is controlled by the apparition of a complex organisation of the landscape that splits into a remarkable hierarchy of minima as jamming is approached. Our results show that the mean-field prediction of a Gardner phase characterized by an ultrametric structure of the landscape provides a useful description of finite dimensional systems, even when the Gardner transition is avoided.
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Can the glass transition be explained without a growing static length scale?
Auteur(s): Berthier L., Biroli Giulio, Bouchaud Jean-Philippe, Tarjus Gilles
(Article) Publié:
The Journal Of Chemical Physics, vol. 150 p.094501 (2019)
Texte intégral en Openaccess :
Ref HAL: hal-02082177_v1
Ref Arxiv: 1805.12378
DOI: 10.1063/1.5086509
WoS: 000460786600023
Ref. & Cit.: NASA ADS
Exporter : BibTex | endNote
19 Citations
Résumé: It was recently discovered that SWAP, a Monte Carlo algorithm that involves the exchange of pairs of particles of differing diameters, can dramatically accelerate the equilibration of simulated supercooled liquids in regimes where the normal dynamics is glassy. This spectacular effect was subsequently interpreted as direct evidence against a static, cooperative explanation of the glass transition such as the one offered by the random first-order transition (RFOT) theory. We review several empirical facts that support the opposite view, namely, that a local mechanism cannot explain the glass transition phenomenology. We explain the speedup induced by SWAP within the framework of the RFOT theory. We suggest that the efficiency of SWAP stems from a postponed onset of glassy dynamics, which allows the efficient exploration of configuration space even in the regime where the physical dynamics is dominated by activated events across free-energy barriers. We describe this effect in terms of `crumbling metastability' and use the example of nucleation to illustrate the possibility of circumventing free-energy barriers of thermodynamic origin by a change of the local dynamical rules.
Commentaires: 15 pages, 3 figures; v2: improved discussions and clarifications
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Towards a coherent picture of the mode-coupling glass crossover
Auteur(s): Coslovich D.
Conférence invité: The Physical Society of Japan 2019 Annual (74th) Meeting (Fukuoka, JP, 2019-03-14)
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Bypassing sluggishness: SWAP algorithm and glassiness in high dimensions
Auteur(s): Berthier L., Charbonneau Patrick, Kundu Joyjit
(Article) Publié:
Physical Review E: Statistical, Nonlinear, And Soft Matter Physics, vol. p.031301 (2019)
Texte intégral en Openaccess :
Ref HAL: hal-02074910_v1
Ref Arxiv: 1810.06950
DOI: 10.1103/PhysRevE.99.031301
WoS: 000460663400001
Ref. & Cit.: NASA ADS
Exporter : BibTex | endNote
8 Citations
Résumé: The recent implementation of a swap Monte Carlo algorithm (SWAP) for polydisperse mixtures fully bypasses computational sluggishness and closes the gap between experimental and simulation timescales in physical dimensions $d=2$ and $3$. Here, we consider suitably optimized systems in $d=2, 3,\dots, 8$, to obtain insights into the performance and underlying physics of SWAP. We show that the speedup obtained decays rapidly with increasing the dimension. SWAP nonetheless delays systematically the onset of the activated dynamics by an amount that remains finite in the limit $d \to \infty$. This shows that the glassy dynamics in high dimensions $d>3$ is now computationally accessible using SWAP, thus opening the door for the systematic consideration of finite-dimensional deviations from the mean-field description.
Commentaires: Réf Journal: Phys. Rev. E 99, 031301 (2019)
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Vibrational properties of sodosilicate glasses from first-principles calculations
Auteur(s): Kilymis D., Ispas S., Hehlen B., Peuget S., Delaye Jean-Marc
(Article) Publié:
Physical Review B, vol. 99 p.054209 (2019)
Texte intégral en Openaccess :
Ref HAL: hal-02043157_v1
DOI: 10.1103/PhysRevB.99.054209
WoS: 000459221700002
Exporter : BibTex | endNote
5 Citations
Résumé: The vibrational properties of three sodosilicate glasses have been investigated in the framework of density functional theory. The pure vibrational density of states has been calculated for all systems and the different vibrational modes have been assigned to specific atoms or structuralunits. It is shown that the Na content affects several vibrational features as the position and intensity of the R band or the mixing of the rocking and bending atomic motions of the Si-O-Si bridges. The calculated Raman spectra have been found to agree with experimental observations and their decomposition indicated the dominant character of the non-bridging oxygen contribution on the spectra, in particular for the high-frequency band, above 800 cm −1 . The decomposition of the high-frequency Raman feature into vibrations of the depolymerized tetrahedra (i.e. Q n -units) has revealed spectral shapes of the partial contributions that cannot be accounted for by simple Gaussians as frequently assumed in the treatment of experimentally obtained Raman spectra.
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Marginally stable phases in mean-field structural glasses
Auteur(s): Scalliet C., Berthier L., Zamponi Francesco
(Article) Publié:
Physical Review E, vol. 99 p.012107 (2019)
Texte intégral en Openaccess :
Ref HAL: hal-02022558_v1
Ref Arxiv: 1810.01213
DOI: 10.1103/PhysRevE.99.012107
WoS: WOS:000455062400003
Ref. & Cit.: NASA ADS
Exporter : BibTex | endNote
11 Citations
Résumé: A novel form of amorphous matter characterized by marginal stability was recently discovered in the mean-field theory of structural glasses. Using this approach, we provide complete phase diagrams delimiting the location of the marginally stable glass phase for a large variety of pair interactions and physical conditions, extensively exploring physical regimes relevant to granular matter, foams, emulsions, hard and soft colloids, and molecular glasses. We find that all types of glasses may become marginally stable, but the extent of the marginally stable phase highly depends on the preparation protocol. Our results suggest that marginal phases should be observable for colloidal and non-Brownian particles near jamming and for poorly annealed glasses. For well-annealed glasses, two distinct marginal phases are predicted. Our study unifies previous results on marginal stability in mean-field models and will be useful to guide numerical simulations and experiments aimed at detecting marginal stability in finite-dimensional amorphous materials.
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How glasses break: A randomcritical point for yielding
Auteur(s): Berthier L.
Conférence invité: Avalanche dynamics and precursors of catastrophic events (Les Houches, FR, 2019-02-04)
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