Ref HAL: hal-00018421_v1
Exporter : BibTex | endNote
Résumé:

Time-resolved carrier dynamics in single wall carbon nanotubes is investigated by means of two-color pump-probe experiments. The recombination dynamics is monitored by probing the transient photo-bleaching observed on the first interband transition of the semi-conducting tubes. The carrier dynamics takes place on a one picosecond time scale which is one order of magnitude slower than in graphite. Transient photo-induced absorption is observed with exactly the same dynamics for non-resonant probe conditions and is interpreted as a global red shift of the $\pi-$plasmon resonance. We show that the opening of the band gap in semi-conducting carbon nanotubes determines the non-linear response dynamics over the whole visible and near-infrared spectrum.